July 11, 2023
Journal Article

Stacked target irradiations and radiochemical separations for simultaneous production of short-lived Ni and Ir isotopes

Abstract

A method was developed for simultaneous production of neutron-deficient Ni and Ir isotopes by irradiation of stacked targets with a 50.5 MeV proton beam, followed by radiochemical separations to remove excess target material. The target, irradiation configuration, and post-irradiation radiochemical separations were developed and tested in a proof-of-principle irradiation. Radiochemical yields and purity of the products are discussed. The stacked target method, developed herein, can be used to produce other isotope pairs with appropriate beam tailoring

Published: July 11, 2023

Citation

Morrison E.C., S.S. Morrison, J.M. Bowen, B.D. Pierson, L.R. Greenwood, V.T. Woods, and C.Z. Soderquist, et al. 2023. Stacked target irradiations and radiochemical separations for simultaneous production of short-lived Ni and Ir isotopes. Journal of Radioanalytical and Nuclear Chemistry 332, no. 2023:2533-2542. PNNL-SA-178600. doi:10.1007/s10967-023-08917-1